收稿：2021-01-25，
纸质出版：2021-06-28
移动端阅览
碳酸盐的团簇同位素（Δ
47
）可以直接确定矿物的形成温度，结合矿物的氧同位素，还可以根据传统的氧同位素温度计确定矿物生长的流体（水）的氧同位素（δ
18
O），提供了一种潜在的确定白云化流体的δ
18
O、分析白云岩化流体来源的新方法。受白云岩化之后的重结晶作用和高温固态重置作用的影响，白云岩的团簇同位素温度（
T
Δ
47
）会比白云化作用实际发生时期的温度偏高，给直接利用
T
Δ
47
来恢复白云岩化流体的δ
18
O造成了一定的局限性。为了分析四川盆地东北部地区长兴组-飞仙关组白云岩化流体的来源，开展了普光气田和元坝气田的白云岩团簇同位素研究。普光气田和元坝气田长兴组-飞仙关组白云岩的
T
Δ
47
在70~130 ℃，是重结晶作用和固态重置之后的白云岩视平衡温度。根据地层温度演化史和白云石的固态重置模型，固态重置作用导致川东北地区白云岩的平衡温度增高了30~35 ℃。经固态重置恢复之后确定的白云化流体的δ
18
O（SMOW）在0~4‰，表明白云岩化流体来源于高盐度的蒸发流体。
Clumped isotopes (Δ
47
) can be used to det
ermine formation temperature of carbonate minerals.If combined with the conventional oxygen thermometer and δ
18
O of the minerals
the temperature can be used further to calculate the δ
18
O of fluids (water)
in which the minerals are developed.This provides a potential new method for determining the δ
18
O and sources of dolomitizing fluids.However
affected by recrystallization and solid-state reordering after dolomitization
the clumped isotope temperature (
T
Δ
47
) usually reads higher than the actual dolomitization temperature
thus limiting the application of
T
Δ
47
to the restoration of fluid δ
18
O.To determine the sources of the dolomitizing fluids from the Changxing (P
2
c
) and Feixianguan Formations (T
1
f
) in northeastern Sichuan Basin
clumped isotopes of dolostone samples from the Puguang and Yuanba gas fields were collected and measured.The
T
Δ
47
of P
2
c
and T
1
f
dolostone samples from the two gas fields ranges between 70 ℃ and 130 ℃
which
however
should be seen as apparent temperature of the samples considering the effect of recrystallization and solid-state reordering.The thermal history and solid-state reordering model results show that the apparent temperature of the samples would increase by about 30-35 ℃ under high-temperature solid-state reordering and the δ
18
O of the dolomitizing fluids is 0-4‰ (SMOW) after restoring solid-state reordering
indicating a high-salinity evaporative sea water source.
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