塔里木盆地天然气中稀有气体地球化学特征

doi:10.11743/ogg20200409

Abstract

Abstract:

The isotopic characteristics of noble gases have been long used in the study of the genesis and origin of natural gases.A systematic analysis of the abundance and isotopic composition of noble gases in natural gases from different structural units shows that the majority of samples is low in the ratio of ³He/⁴He, with the R/R_a values generally less than 0.1, indicating a crustal radiogenic genesis of the noble gases and a significant "cold" feature of the basin.No simple correlation exists between the ³He/⁴He ratios and both of heat flow and paleo-geothermal gradient, revealing little heat sourcing from mantle.The lower level of ²¹Ne/²²Ne ratios influenced by the relatively late hydrocarbon generation and accumulation period, mostly during the Himalaya movement, shows an inconspicuous proportion of mantle-derived gas in natural gases from Kuqa Depression.The relative depletion of ¹²⁹Xe shows that the mixing of mantle-derived volatile constituents is insignificant.Furthermore, compared with the natural gases from Tabei Uplift and Tazhong Uplift, the Xe in natural gases from Kuqa Depression was more likely derived from the crust due to the influences of lithology and structural features.

Key words: mantle-derived, terrestrial heat flow, isotope, noble gas, natural gas, Kuqa Depression, Tarim Basin

CLC Number:

TE122.1

Daxiang He, Youjun Tang, Jinjie Hu, Shaowu Mo, Jianfa Chen. Geochemical characteristics of noble gases in natural gases from the Tarim Basin[J]. Oil & Gas Geology, 2020, 41(4): 755-762.

Figures/Tables 9

Fig.1

Table 1

Constituents and isotopes of noble gases in natural gases from the Tarim Basin"

井号	层位	深度/m	稀有气体组分含量/10^-6					³He/⁴He(10^-6)	R/R_a	Ar/He	⁴⁰Ar/³⁶Ar	¹²⁹Xe/¹³⁰Xe	¹³²Xe/¹³⁰Xe	¹³⁶Xe/¹³⁰Xe
井号	层位	深度/m	He	Ne	Ar	Kr	Xe	³He/⁴He(10^-6)	R/R_a	Ar/He	⁴⁰Ar/³⁶Ar	¹²⁹Xe/¹³⁰Xe	¹³²Xe/¹³⁰Xe	¹³⁶Xe/¹³⁰Xe
大北302	K	7 209~7 244	58.59	1.98	28.67	0.008 9	0.001 933	0.087	0.062	0.489	504.322	6.388	6.791	2.328
大北201	K	5 932~6 145	49.15	3.97	20.20	0.008 2	0.003 815	0.063	0.045	0.411	858.128	6.446	6.792	2.180
克拉2-1	K	3 675~3 705	40.47	3.34	192.70	0.506 6	0.001 665	0.043	0.031	4.761	1 323.026	6.419	6.792	2.121
克深8	K	6 717~6 795	30.97	2.25	165.90	0.296 8	0.001 551	0.049	0.035	5.357	1 092.812	6.412	6.870	2.355
克深206	K	6 525~6 800	34.87	2.05	30.39	0.003 8	0.001 223	0.050	0.036	0.872	841.061	6.381	6.620	2.334
玉东101	E	4 958~4 970	206.87	5.09	73.22	0.023 5	0.004 712	0.057	0.041	0.354	674.431	6.502	6.775	2.269
玉东6	E	4 745~4 751	200.61	4.97	66.06	0.023 8	0.004 580	0.057	0.041	0.329	606.577	6.251	6.690	2.333
轮古3-2	O	5 180~5 208	170.83	4.72	65.72	0.025 4	0.004 209	0.042	0.030	0.385	555.512	6.388	6.845	2.385
哈901-2	O	6 488~6 670	159.92	4.61	75.21	0.030 3	0.004 771	0.017	0.012	0.470	406.489	6.457	6.737	2.265
热普3	O	6 977~7 040	285.26	6.50	66.50	0.028 6	0.005 667	0.019	0.014	0.233	452.329	6.345	6.712	2.355
塔中83-H5	O	5 314~5 966	232.59	5.07	22.73	0.007 6	0.002 658	0.079	0.057	0.098	844.756	—	—	—
塔中62-13H	O	4 797~5 370	328.49	5.90	27.08	0.008 7	0.003 061	0.031	0.022	0.082	978.664	—	—	—
塔中26-8	O	4 266~5 029	550.27	10.29	72.10	0.029 7	0.008 254	0.014	0.010	0.131	886.558	6.261	6.846	2.306
塔中82-TH	O	5 335~5 632	433.67	8.61	55.88	0.026 3	0.006 612	0.048	0.034	0.129	906.359	6.405	6.973	2.263
塔中4-6-21H	C	3 612~3 623	596.09	12.23	172.35	0.043 5	0.010 455	0.043	0.031	0.289	773.850	6.477	6.656	2.352
中古111	O	6 008~6 250	96.06	4.87	10.24	0.010 6	0.006 291	0.040	0.028	0.107	685.175	6.314	6.733	2.358
中古43	O	4 980~5 334	305.87	6.84	43.90	0.013 4	0.004 443	0.072	0.051	0.144	658.639	6.477	6.711	2.236
中深1C		6 861~6 944	751.90	14.75	204.72	0.042 6	0.011 375	0.081	0.058	0.272	3 745.175	6.462	6.873	2.221
中古17	O	6 206~6 448	288.83	6.29	40.83	0.011 5	0.003 521	0.045	0.032	0.141	836.078	6.293	6.777	2.305
中古6	O	5 934~6 172	331.44	6.85	73.25	0.023 1	0.004 962	0.077	0.055	0.221	860.241	—	—	—
中古21	O	5 753~5 874	158.78	4.19	17.74	0.006 8	0.002 150	0.037	0.027	0.112	658.120	—	—	—
玛4-H1	C	1 931~2 433	1 839.04	31.06	415.88	0.078 0	0.023 028	0.106	0.076	0.226	2 039.713	6.407	6.643	2.317
大气	—	—	5.25	18.18	9 340.00	1.140 0	0.008 700	1.400	—	1 782.443	295.500	6.496	6.607	2.176

Table 1

Fig.2

Fig.3

Fig.4

Fig.5

Fig.6

Fig.7

Fig.8

References 30

1	魏国齐, 王东良, 王晓波, 等. 四川盆地高石梯-磨溪大气田稀有气体特征[J]. 石油勘探与开发, 2014, 41 (5): 533- 538.
	Wei Guoqi , Wang Dongliang , Wang Xiaobo , et al. Characteristics of noble gases in the large Gaoshiti-Moxi gas field in Sichuan Basin[J]. Petroleum Exploration and Development, 2014, 41 (5): 533- 538.
2	戴金星, 李剑, 侯路. 鄂尔多斯盆地氦同位素的特征[J]. 高校地质学报, 2005, 11 (4): 473- 478. doi: 10.3969/j.issn.1006-7493.2005.04.002
	Dai Jinxing , Li Jian , Hou Lu . Characteristics of helium isotopes in the Ordos Basin[J]. Geological Journal of China Universities, 2005, 11 (4): 473- 478. doi: 10.3969/j.issn.1006-7493.2005.04.002
3	Wang X B , Wei G Q , Li J , et al. Geochemical characteristics and origins of noble gases of the Kela 2 gas field in the Tarim Basin, China[J]. Marine and Petroleum Geology, 2018, 89, 155- 163. doi: 10.1016/j.marpetgeo.2017.02.013
4	陈践发, 王万春, 朱岳年. 含油气盆地中天然气汞含量的主要影响因素[J]. 石油与天然气地质, 2001, 22 (4): 352- 354. doi: 10.3321/j.issn:0253-9985.2001.04.014
	Chen Jianfa , Wang Wanchun , Zhu Yuenian . Affecting factors of hg contents in gases in petroliferous basins[J]. Oil & Gas Geology, 2001, 22 (4): 352- 354. doi: 10.3321/j.issn:0253-9985.2001.04.014
5	朱铭. 天然气藏中氩同位素积累模式及其定年公式[J]. 地质科学, 1990, (2): 166- 172.
	Zhu Ming . A model for accumulation of isotopic composition in natural gas and its application to dating[J]. Scientia Geologica Sinica, 1990, (2): 166- 172.
6	刘文汇, 孙明良, 徐永昌. 鄂尔多斯盆地天然气稀有气体同位素特征及气源示踪[J]. 科学通报, 2001, 46 (22): 1902- 1905. doi: 10.3321/j.issn:0023-074X.2001.22.014
	Liu Wenhui , Sun Mingliang , Xu Yongchang . Isotopic characteristics of noble gases in natural gases from Ordos basin and souce trace[J]. Chinese Science Bulletin, 2001, 46 (22): 1902- 1905. doi: 10.3321/j.issn:0023-074X.2001.22.014
7	徐胜, 徐永昌, 沈平, 等. 中国东部盆地天然气中氖同位素组成及其地质意义[J]. 科学通报, 1996, 41 (21): 1970- 1972. doi: 10.3321/j.issn:0023-074X.1996.21.013
	Xu Sheng , Xu Yongchang , Shen Ping , et al. Ne isotopes in natural gases from basins in eastern China and its geological significance[J]. Chinese Science Bulletin, 1996, 41 (21): 1970- 1972. doi: 10.3321/j.issn:0023-074X.1996.21.013
8	Byrne D J , Barry P H , Lawson M , et al. Determining gas expulsion vs retention during hydrocarbon generation in the Eagle Ford Shale using noble gases[J]. Geochimica et Cosmochimica Acta, 2018, (241): 240- 254.
9	贾承造. 中国塔里木盆地构造特征与油气[M]. 北京: 石油工业出版社, 1997: 1- 5.
	Jia Chengzao Caineng . Tectonic characteristics and petroleum, Tarim Basin China[M]. Beijing: Petroleum Industry Press, 1997: 1- 5.
10	张水昌, 梁狄刚, 张宝民, 等. 塔里木盆地海相油气的生成[M]. 北京: 石油工业出版社, 2004: 55- 76.
	Zhang Shuichang , Liang Digang , Zhang Baoming , et al. Marine hydrocarbon generating of Tarim[M]. Beijing: Petroleum Industry Press, 2004: 55- 76.
11	赵靖舟. 塔里木盆地油气藏形成与分布规律[M]. 北京: 石油工业出版社, 2003: 60- 86.
	Zhao Jingzhou . The formation and distribution of reservoirs in Tarim basin[M]. Beijing: Petroleum Industry Press, 2003: 60- 86.
12	苏洲, 张慧芳, 韩剑发, 等. 塔里木盆地库车坳陷中、新生界高蜡凝析油和轻质油形成及其控制因素[J]. 石油与天然气地质, 2018, 39 (6): 1255- 1269.
	Su Zhou , Zhang Huifang , Han Jianfa , et al. Origin and controlling factors of Mesozoic-Cenozoic gas condensates with high wax content and high-gravity oil in Kuqa Depression[J]. Oil & Gas Geology, 2018, 39 (6): 1255- 1269.
13	鲜强, 冯许魁, 刘永雷, 等. 塔中地区碳酸盐岩缝洞型储层叠前流体识别[J]. 石油与天然气地质, 2019, 40 (01): 196- 204.
	Xian Qiang , Feng Xukui , Liu Yonglei , et al. Pre-stack fluid identification for fractured-vuggy carbonate reservoir in Tazhong area[J]. Oil & Gas Geology, 2019, 40 (1): 196- 204.
14	田亮, 李佳玲, 袁飞宇, 等. 塔河油田碳酸盐岩缝洞型油藏定量化注水技术研究[J]. 石油地质与工程, 2018, 32 (2): 86- 89. doi: 10.3969/j.issn.1673-8217.2018.02.023
	Tian Liang , Li Jialing , Yuan Feiyu , et al. Quantitative water injection of fractured-cavity oil reservoir in carbonate rocks in Tahe oilfield[J]. Petroleum Geology & Engineering, 2018, 32 (2): 86- 89. doi: 10.3969/j.issn.1673-8217.2018.02.023
15	贾承造. 塔里木盆地板块构造与大陆动力学[M]. 北京: 石油工业出版社, 2004: 149- 166.
	Jia Chengzao . Plate tectonics and continental dynamics, Tarim Basin[M]. Beijing: Petroleum Industry Press, 2004: 149- 166.
16	王玉伟, 陈红汉, 郭会芳, 等. 塔里木盆地顺1走滑断裂带超深储层油气充注历史[J]. 石油与天然气地质, 2019, 40 (05): 972- 989.
	Wang Yuwei , Chen Honghan , Guo Hhuifang , et al. Hydrocarbon charging history of the ultra-deep reservoir in Shun 1strike-slip fault zone[J]. Oil & Gas Geology, 2019, 40 (5): 972- 989.
17	徐永昌, 沈平, 刘文汇, 等. 天然气中稀有气体地球化学[M]. 北京: 科学出版社, 1998: 74- 91.
	Xu Yongchang , Shen Ping , Liu Wenhui , et al. Noble gas geochemistry in natural gases[M]. Beijing: Science Press, 1998: 74- 91.
18	杜建国, 徐永昌, 孙明良. 中国大陆含油气盆地的氦同位素组成及大地热流密度[J]. 地球物理学报, 1998, 41 (4): 494- 501. doi: 10.3321/j.issn:0001-5733.1998.04.008
	Du Jianguo , Xu Yongchang , Sun Mingliang . Helium isotopes and heat flow in the oil and gas bearing basins in China's continent[J]. Acta Geophysica Sinica, 1998, 41 (4): 494- 501. doi: 10.3321/j.issn:0001-5733.1998.04.008
19	汪集暘, 邱楠生, 胡圣标, 等. 中国油田地热研究的进展和发展趋势[J]. 地学前缘, 2017, 24 (3): 1- 12.
	Wang Jiyang , Qiu Nansheng , Hu Shengbiao , et al. Advancement and developmental trend in the geothermics of oil fields in China[J]. Earth Science Frontiers, 2017, 24 (3): 1- 12.
20	陈汉林, 杨树锋, 董传万, 等. 塔里木盆地地质热事件研究[J]. 科学通报, 1997, 42 (10): 1096- 1099. doi: 10.3321/j.issn:0023-074X.1997.10.021
	Chen Hanlin , Yang Shufeng , Dong Chuanwan , et al. The research on the thermal events in Tarim Basin[J]. Chinese Science Bulletin, 1997, 42 (10): 1096- 1099. doi: 10.3321/j.issn:0023-074X.1997.10.021
21	王良书, 李成. 塔里木盆地大地热流密度分布特征[J]. 地球物理学报, 1995, 38 (6): 855- 856. doi: 10.3321/j.issn:0001-5733.1995.06.019
	Wang Liangshu , Li Chen . Distribution of terrestrial heat flow density in Tarim Basin, western China[J]. Acta Geophysica Sinica, 1995, 38 (6): 855- 856. doi: 10.3321/j.issn:0001-5733.1995.06.019
22	刘绍文, 李香兰, 郝春艳, 等. 塔里木盆地的热流、深部温度和热结构[J]. 地学前缘, 2017, 24 (3): 41- 55.
	Liu Shaowen , Li Xianglan , Hao Chunyan , et al. Heat flow, deep formation temperature and thermal structure of the Tarim Basin, Northwest China[J]. Earth Science Frontiers, 2017, 24 (3): 41- 55.
23	张秋茶, 王福焕, 肖中尧, 等. 阿克1井天然气气源探讨[J]. 天然气地球科学, 2003, 14 (6): 484- 487. doi: 10.3969/j.issn.1672-1926.2003.06.012
	Zhang Qiucha , Wang Fuhuan , Xiao Zhongyao , et al. The discussion of natural gas source in well Ake 1[J]. Natural Gas Geoscience, 2003, 14 (6): 484- 487. doi: 10.3969/j.issn.1672-1926.2003.06.012
24	Ballentine C J , O'nions R K , Coleman M L . A magnus opus:Helium, neon, and argon isotopes in a North Sea oilfield[J]. Geochimica et Cosmochimica Acta, 1996, 60 (5): 831- 849. doi: 10.1016/0016-7037(95)00439-4
25	Xu S , Nakai S , Wakita H , et al. Mantle-derived noble gases in natural gases from Songliao Basin, China[J]. Geochimica et Cosmochimica Acta, 1995, 59 (22): 4675- 4683. doi: 10.1016/0016-7037(95)00301-0
26	李丕龙, 冯建辉, 樊太亮, 等. 塔里木盆地构造沉积与成藏[M]. 2010,北京: 地质出版社, 2010: 212- 233.
	Li Pilong , Feng Jianhui , Fan Tailiang , et al. Tectonic-sedimentary evolution and hydrocarbon accumulation of Tarim Basin[M]. Beijing: Geological Press, 2010: 212- 233.
27	郑见超, 李斌, 刘羿伶, 等. 塔里木盆地下寒武统玉尔吐斯组烃源岩热演化模拟分析[J]. 油气藏评价与开发, 2018, 8 (6): 7- 12. doi: 10.3969/j.issn.2095-1426.2018.06.002
	Zheng Jianchao , Li Bin , Liu Yiling , et al. Study on thermal evolution modeling of lower Cambrian Yuertusi source rock, Tarim Basin[J]. Reservoir Evaluation and Development, 2018, 8 (6): 7- 12. doi: 10.3969/j.issn.2095-1426.2018.06.002
28	徐胜, 徐永昌, 沈平, 等. 中国东部盆地天然气中氙同位素过剩[J]. 科学通报, 1997, 42 (1): 78- 80.
	Xu Sheng , Xu Yongchang , Shen Ping , et al. Excess Xenon in natural gases from basins in eastern China[J]. Chinese Science Bulletin, 1997, 42 (1): 78- 80.
29	刘春花, 吴才来, 郜源红, 等. 南天山拜城县波孜果尔A型花岗岩类锆石U-Pb定年及其Lu-Hf同位素组成[J]. 岩石学报, 2014, 30 (6): 1595- 1614.
	Liu Chunhua , Wu Cailai , Gao Yuanhong , et al. Zircon LA-ICP-MS U-Pb dating and Lu-Hf isotopic system of A-type granitoids in South Tianshan, Baicheng County, Xinjiang[J]. Acta Petrologica Sinica, 30 (6): 1595- 1614.
30	何登发, 李德生, 何金有, 等. 塔里木盆地库车坳陷和西南坳陷油气地质特征类比及勘探启示[J]. 石油学报, 2013, 34 (2): 201- 218.
	He Dengfa , Li Desheng , He Jinyou , et al. Comparison in petroleum geology between Kuqa depression and Southwest depression in Tarin Basin and its exploration significance[J]. Acta Petrolei Sinica, 2013, 34 (2): 201- 218.

[1]	Pengyuan HAN, Wenlong DING, Debin YANG, Juan ZHANG, Hailong MA, Shenghui WANG. Characteristics of the S80 strike-slip fault zone and its controlling effects on the Ordovician reservoirs in the Tahe oilfield， Tarim Basin [J]. Oil & Gas Geology, 2024, 45(3): 770-786.
[2]	Yanqiu ZHANG, Honghan CHEN, Xiepei WANG, Peng WANG, Danmei SU, Zhou XIE. Assessment of connectivity between source rocks and strike-slip fault zone in the Fuman oilfield， Tarim Basin [J]. Oil & Gas Geology, 2024, 45(3): 787-800.
[3]	Wenlong DING, Yuntao LI, Jun HAN, Cheng HUANG, Laiyuan WANG, Qingxiu MENG. Methods for high-precision tectonic stress field simulation and multi-parameter prediction of fracture distribution for carbonate reservoirs and their application [J]. Oil & Gas Geology, 2024, 45(3): 827-851.
[4]	Zicheng CAO, Lu YUN, Lixin QI, Haiying LI, Jun HAN, Feng GENG, Bo LIN, Jingping CHEN, Cheng HUANG, Qingyan MAO. A major discovery of hydrocarbon-bearing layers over 1，000-meter thick in well Shunbei 84X， Shunbei area， Tarim Basin and its implications [J]. Oil & Gas Geology, 2024, 45(2): 341-356.
[5]	Debin YANG, Xinbian LU, Dian BAO, Fei CAO, Yan WANG, Ming WANG, Runcheng XIE. New insights into the genetic types and characteristics of the Ordovician marine fault-karst carbonate reservoirs in the northern Tarim Basin [J]. Oil & Gas Geology, 2024, 45(2): 357-366.
[6]	Changjian ZHANG, Debin YANG, Lin JIANG, Yingbing JIANG, Qi CHANG, Xuejian MA. Characteristics and origin of over-dissolution residual fault-karst reservoirs in the northern Tahe oilfield， Tarim Basin [J]. Oil & Gas Geology, 2024, 45(2): 367-383.
[7]	Chenglin LIU, Zhengang DING, Liyong FAN, Rui KANG, Sijie HONG, Yuxin ZHU, Jianfa CHEN, Haidong WANG, Nuo XU. Geochemical characteristics and enrichment factors of helium-bearing natural gas in the Ordos Basin [J]. Oil & Gas Geology, 2024, 45(2): 384-392.
[8]	Tongwen JIANG, Xingliang DENG, Peng CAO, Shaoying CHANG. Storage space types and water-flooding efficiency for fault-controlled fractured oil reservoirs in Fuman oilfield， Tarim Basin [J]. Oil & Gas Geology, 2024, 45(2): 542-552.
[9]	Mingxing BAI, Zhichao ZHANG, Qiaozhen CHEN, Long XU, Siyu DU, Yexin LIU. Advances in research on CO₂ replacement for natural gas hydrate exploitation [J]. Oil & Gas Geology, 2024, 45(2): 553-564.
[10]	Lidong MI, Daqian ZENG, Hua LIU, Yandong GUO, Yanfeng LI, Zunzhao LI, Xudong SUN, Guangquan ZHANG, Chunhua LU, Peixian WANG. Key technologies and development trends for intelligent construction of underground gas storage facilities [J]. Oil & Gas Geology, 2024, 45(2): 581-592.
[11]	Yuemeng NIU, Jun HAN, Yixin YU, Cheng Huang, Bo Lin, Fan YANG, Lang YU, Junyu CHEN. Igneous rock intrusions in the western Shunbei area， Tarim Basin： Characteristics and coupling relationships with faults [J]. Oil & Gas Geology, 2024, 45(1): 231-242.
[12]	Chenglin LIU, Zhengang DING, Jianfa CHEN, Liyong FAN, Rui KANG, Haidong WANG, Sijie HONG, Anqi TIAN, Xueyong CHEN. Characteristics and helium-generating potential of helium source rocks in the Ordos Basin [J]. Oil & Gas Geology, 2023, 44(6): 1546-1554.
[13]	San ZHANG, Qiang JIN, Jinxiong SHI, Mingyi HU, Mengyue DUAN, Yongqiang LI, Xudong ZHANG, Fuqi CHENG. Filling patterns and reservoir property of the Ordovician buried-river karst caves in the Tabei area， Tarim Basin [J]. Oil & Gas Geology, 2023, 44(6): 1582-1594.
[14]	Zhiyong GAO, Yongping WU, Zhaolong LIU, Cong WEI, Yongzhong ZHANG, Cuili WANG, Qunming LIU. Development model and significance of favorable lithofacies association of sandy braided river facies of the Cretaceous Bashijiqike Formation in Zhongqiu 1 well block， Kuqa Depression， Tarim Basin [J]. Oil & Gas Geology, 2023, 44(5): 1141-1158.
[15]	Han LI, Jinhua FU, Hancheng JI, Lei ZHANG, Yuwei SHE, Wei GUAN, Xianghui JING, Hongwei WANG, qian CAO, Gang LIU, Jiayi WEI. Bauxite series in the Upper Paleozoic weathering crusts in the southwestern Ordos Basin： Development and distribution of dominant reservoirs [J]. Oil & Gas Geology, 2023, 44(5): 1243-1255.

Geochemical characteristics of noble gases in natural gases from the Tarim Basin

RichHTML

PDF (PC)

Knowledge

Abstract

Cite this article

share this article

Figures/Tables 9

References 30

Related Articles 15

Recommended Articles

Metrics