塔里木盆地天然气中稀有气体地球化学特征

doi:10.11743/ogg20200409

石油与天然气地质 ›› 2020, Vol. 41 ›› Issue (4): 755-762.doi: 10.11743/ogg20200409

塔里木盆地天然气中稀有气体地球化学特征

何大祥^1,^2,³(), 唐友军^1,², 胡锦杰^1,², 莫少武^1,², 陈践发^3,*()

1. 长江大学油气资源与勘探技术教育部重点实验室, 湖北武汉 430100
2. 长江大学资源与环境学院, 湖北武汉 430100
3. 中国石油大学(北京) 地球科学学院油气资源与探测国家重点实验室, 北京 102249

收稿日期:2018-12-21 出版日期:2020-08-01 发布日期:2020-08-11
通讯作者: 陈践发 E-mail:hedaxiang127@163.com;jfchen@cup.edu.cn
第一作者简介:何大祥(1986—)，男，博士、讲师，油气地球化学。E-mail:hedaxiang127@163.com
基金项目:
中国石油科技创新基金项目(2017D-5007-0105);油气资源与探测国家重点实验室开放基金项目(PRP/open-1710);油气资源与勘探技术教育部重点实验室（长江大学）开放基金项目(K2018-20)

Geochemical characteristics of noble gases in natural gases from the Tarim Basin

Daxiang He^1,^2,³(), Youjun Tang^1,², Jinjie Hu^1,², Shaowu Mo^1,², Jianfa Chen^3,*()

1. Key Laboratory of Oil and Gas Resources and Exploration Technology(Yangtze University), Ministry of Education, Wuhan, Hubei 430100, China
2. College of Resources and Environment, Yangtze University, Wuhan, Hubei 430100, China
3. State Key Laboratory of Petroleum Resources and Prospecting, College of Geosciences, China University of Petroleum(Beijing), Beijing 102249, China

Received:2018-12-21 Online:2020-08-01 Published:2020-08-11
Contact: Jianfa Chen E-mail:hedaxiang127@163.com;jfchen@cup.edu.cn

摘要/Abstract

摘要：

利用天然气中稀有气体同位素组成特征可以有效地判识天然气的成因和来源。塔里木盆地不同构造单元典型天然气藏天然气中稀有气体丰度和同位素组成分析表明，天然气样品的³He/⁴He值均普遍较低，R/R_a值均小于0.1，天然气中的稀有气体主要为壳源放射性成因，指示低温“冷盆”的特征。³He/⁴He组成与热流值和古地温梯度之间没有简单的对应关系，指示盆地地幔热的来源较少。库车坳陷天然气成藏时代较晚，多为喜马拉雅期，其²¹Ne/²²Ne较低，反映其受地幔端元混染作用较小。天然气中¹²⁹Xe相对亏损，指示无明显的幔源挥发分的混入，受岩性及构造特征的影响，相较于塔北隆起、塔中隆起天然气，库车坳陷天然气中Xe的壳源特征更为明显。

关键词: 幔源, 大地热流, 同位素, 稀有气体, 天然气, 库车坳陷, 塔里木盆地

Abstract:

The isotopic characteristics of noble gases have been long used in the study of the genesis and origin of natural gases.A systematic analysis of the abundance and isotopic composition of noble gases in natural gases from different structural units shows that the majority of samples is low in the ratio of ³He/⁴He, with the R/R_a values generally less than 0.1, indicating a crustal radiogenic genesis of the noble gases and a significant "cold" feature of the basin.No simple correlation exists between the ³He/⁴He ratios and both of heat flow and paleo-geothermal gradient, revealing little heat sourcing from mantle.The lower level of ²¹Ne/²²Ne ratios influenced by the relatively late hydrocarbon generation and accumulation period, mostly during the Himalaya movement, shows an inconspicuous proportion of mantle-derived gas in natural gases from Kuqa Depression.The relative depletion of ¹²⁹Xe shows that the mixing of mantle-derived volatile constituents is insignificant.Furthermore, compared with the natural gases from Tabei Uplift and Tazhong Uplift, the Xe in natural gases from Kuqa Depression was more likely derived from the crust due to the influences of lithology and structural features.

Key words: mantle-derived, terrestrial heat flow, isotope, noble gas, natural gas, Kuqa Depression, Tarim Basin

中图分类号:

TE122.1

何大祥,唐友军,胡锦杰,等. 塔里木盆地天然气中稀有气体地球化学特征[J]. 石油与天然气地质, 2020, 41(4): 755-762. doi: 10.11743/ogg20200409 Daxiang He,Youjun Tang,Jinjie Hu,et al. Geochemical characteristics of noble gases in natural gases from the Tarim Basin[J]. Oil & Gas Geology, 2020, 41(4): 755-762. doi: 10.11743/ogg20200409

图/表 9

图1

表1

塔里木盆地天然气中稀有气体组分及同位素数据"

井号	层位	深度/m	稀有气体组分含量/10^-6					³He/⁴He(10^-6)	R/R_a	Ar/He	⁴⁰Ar/³⁶Ar	¹²⁹Xe/¹³⁰Xe	¹³²Xe/¹³⁰Xe	¹³⁶Xe/¹³⁰Xe
井号	层位	深度/m	He	Ne	Ar	Kr	Xe	³He/⁴He(10^-6)	R/R_a	Ar/He	⁴⁰Ar/³⁶Ar	¹²⁹Xe/¹³⁰Xe	¹³²Xe/¹³⁰Xe	¹³⁶Xe/¹³⁰Xe
大北302	K	7 209~7 244	58.59	1.98	28.67	0.008 9	0.001 933	0.087	0.062	0.489	504.322	6.388	6.791	2.328
大北201	K	5 932~6 145	49.15	3.97	20.20	0.008 2	0.003 815	0.063	0.045	0.411	858.128	6.446	6.792	2.180
克拉2-1	K	3 675~3 705	40.47	3.34	192.70	0.506 6	0.001 665	0.043	0.031	4.761	1 323.026	6.419	6.792	2.121
克深8	K	6 717~6 795	30.97	2.25	165.90	0.296 8	0.001 551	0.049	0.035	5.357	1 092.812	6.412	6.870	2.355
克深206	K	6 525~6 800	34.87	2.05	30.39	0.003 8	0.001 223	0.050	0.036	0.872	841.061	6.381	6.620	2.334
玉东101	E	4 958~4 970	206.87	5.09	73.22	0.023 5	0.004 712	0.057	0.041	0.354	674.431	6.502	6.775	2.269
玉东6	E	4 745~4 751	200.61	4.97	66.06	0.023 8	0.004 580	0.057	0.041	0.329	606.577	6.251	6.690	2.333
轮古3-2	O	5 180~5 208	170.83	4.72	65.72	0.025 4	0.004 209	0.042	0.030	0.385	555.512	6.388	6.845	2.385
哈901-2	O	6 488~6 670	159.92	4.61	75.21	0.030 3	0.004 771	0.017	0.012	0.470	406.489	6.457	6.737	2.265
热普3	O	6 977~7 040	285.26	6.50	66.50	0.028 6	0.005 667	0.019	0.014	0.233	452.329	6.345	6.712	2.355
塔中83-H5	O	5 314~5 966	232.59	5.07	22.73	0.007 6	0.002 658	0.079	0.057	0.098	844.756	—	—	—
塔中62-13H	O	4 797~5 370	328.49	5.90	27.08	0.008 7	0.003 061	0.031	0.022	0.082	978.664	—	—	—
塔中26-8	O	4 266~5 029	550.27	10.29	72.10	0.029 7	0.008 254	0.014	0.010	0.131	886.558	6.261	6.846	2.306
塔中82-TH	O	5 335~5 632	433.67	8.61	55.88	0.026 3	0.006 612	0.048	0.034	0.129	906.359	6.405	6.973	2.263
塔中4-6-21H	C	3 612~3 623	596.09	12.23	172.35	0.043 5	0.010 455	0.043	0.031	0.289	773.850	6.477	6.656	2.352
中古111	O	6 008~6 250	96.06	4.87	10.24	0.010 6	0.006 291	0.040	0.028	0.107	685.175	6.314	6.733	2.358
中古43	O	4 980~5 334	305.87	6.84	43.90	0.013 4	0.004 443	0.072	0.051	0.144	658.639	6.477	6.711	2.236
中深1C		6 861~6 944	751.90	14.75	204.72	0.042 6	0.011 375	0.081	0.058	0.272	3 745.175	6.462	6.873	2.221
中古17	O	6 206~6 448	288.83	6.29	40.83	0.011 5	0.003 521	0.045	0.032	0.141	836.078	6.293	6.777	2.305
中古6	O	5 934~6 172	331.44	6.85	73.25	0.023 1	0.004 962	0.077	0.055	0.221	860.241	—	—	—
中古21	O	5 753~5 874	158.78	4.19	17.74	0.006 8	0.002 150	0.037	0.027	0.112	658.120	—	—	—
玛4-H1	C	1 931~2 433	1 839.04	31.06	415.88	0.078 0	0.023 028	0.106	0.076	0.226	2 039.713	6.407	6.643	2.317
大气	—	—	5.25	18.18	9 340.00	1.140 0	0.008 700	1.400	—	1 782.443	295.500	6.496	6.607	2.176

表1

图2

图3

图4

图5

图6

图7

图8

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塔里木盆地天然气中稀有气体地球化学特征

Geochemical characteristics of noble gases in natural gases from the Tarim Basin

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