团簇同位素在白云岩化流体恢复中的应用与局限性

doi:10.11743/ogg20210318

摘要/Abstract

摘要：

碳酸盐的团簇同位素（Δ₄₇）可以直接确定矿物的形成温度，结合矿物的氧同位素，还可以根据传统的氧同位素温度计确定矿物生长的流体（水）的氧同位素（δ¹⁸O），提供了一种潜在的确定白云化流体的δ¹⁸O、分析白云岩化流体来源的新方法。受白云岩化之后的重结晶作用和高温固态重置作用的影响，白云岩的团簇同位素温度（T_Δ₄₇）会比白云化作用实际发生时期的温度偏高，给直接利用T_Δ₄₇来恢复白云岩化流体的δ¹⁸O造成了一定的局限性。为了分析四川盆地东北部地区长兴组-飞仙关组白云岩化流体的来源，开展了普光气田和元坝气田的白云岩团簇同位素研究。普光气田和元坝气田长兴组-飞仙关组白云岩的T_Δ₄₇在70~130 ℃，是重结晶作用和固态重置之后的白云岩视平衡温度。根据地层温度演化史和白云石的固态重置模型，固态重置作用导致川东北地区白云岩的平衡温度增高了30~35 ℃。经固态重置恢复之后确定的白云化流体的δ¹⁸O（SMOW）在0~4‰，表明白云岩化流体来源于高盐度的蒸发流体。

关键词: 团簇同位素, 氧同位素, 重结晶作用, 白云岩, 白云岩化流体, 碳酸盐岩, 四川盆地

Abstract:

Clumped isotopes (Δ₄₇) can be used to determine formation temperature of carbonate minerals.If combined with the conventional oxygen thermometer and δ¹⁸O of the minerals, the temperature can be used further to calculate the δ¹⁸O of fluids (water), in which the minerals are developed.This provides a potential new method for determining the δ¹⁸O and sources of dolomitizing fluids.However, affected by recrystallization and solid-state reordering after dolomitization, the clumped isotope temperature (T_Δ₄₇) usually reads higher than the actual dolomitization temperature, thus limiting the application of T_Δ₄₇ to the restoration of fluid δ¹⁸O.To determine the sources of the dolomitizing fluids from the Changxing (P₂c) and Feixianguan Formations (T₁f) in northeastern Sichuan Basin, clumped isotopes of dolostone samples from the Puguang and Yuanba gas fields were collected and measured.The T_Δ₄₇ of P₂c and T₁f dolostone samples from the two gas fields ranges between 70 ℃ and 130 ℃, which, however, should be seen as apparent temperature of the samples considering the effect of recrystallization and solid-state reordering.The thermal history and solid-state reordering model results show that the apparent temperature of the samples would increase by about 30-35 ℃ under high-temperature solid-state reordering and the δ¹⁸O of the dolomitizing fluids is 0-4‰ (SMOW) after restoring solid-state reordering, indicating a high-salinity evaporative sea water source.

Key words: clumped isotope, oxygen isotope, recrystallization, dolostone, dolomitizing fluid, carbonate, Sichuan Basin

中图分类号:

TE122.2

李平平,王淳,邹华耀,等. 团簇同位素在白云岩化流体恢复中的应用与局限性[J]. 石油与天然气地质, 2021, 42(3): 738-746. doi: 10.11743/ogg20210318 Pingping Li,Chun Wang,Huayao Zou,et al. Application of clumped isotopes to restoration of dolomitizing fluids and its limitations[J]. Oil & Gas Geology, 2021, 42(3): 738-746. doi: 10.11743/ogg20210318

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